Investigation of coherent microscopic defects inside the tunneling barrier of a Josephson junction


Book Description

In disordered solids, two-level atomic-tunneling systems are present in large quantity. Only recently, superconducting qubits opened a door for a detection and individual coherent manipulation of such microscopic quantum systems. We succeeded to tune the resonance frequencies of these systems by applying external strain on the qubit chip. Moreover, we observed and analyzed the interaction between two coupled tunneling systems.




Local Investigation of Single Magnetic Molecules with Scanning Tunneling Microscopy


Book Description

We worked on different magnetic molecules containing 3d and 4f magnetic centers. Their growth on metallic surfaces, topographies, spin states, magnetic properties and electron transport were locally investigated by using scanning tunneling microscopy (STM) at temperatures down to 30mK. The main achievement of this dissertation reveals the abrupt switching of crystal fields during formation of molecular contacts.




Investigation of Magnetic Adatoms with Scanning Tunneling Techniques


Book Description

In this work, magnetic atoms on surfaces are studied with low-temperature scanning tunneling microscopy. Motivated by the idea to use single atoms as magnetic bits, the factors that allow or prevent long-term stability of their magnetic moments are investigated. Lifetimes of up to several minutes can be achieved for the magnetic moments of holmium atoms on a Pt(111) surface, resulting from the combined symmetries of the system. Corresponding theoretical calculations are presented and evaluated.







Towards magnetic resonance in scanning tunneling microscopy using heterodyne detection


Book Description

The present work introduces a new concept for magnetic resonance measurements in the GHz regime inside a scanning tunneling microscope. It is based on heterodyne detection in a spin-polarized tunneling barrier. The experimental requirements, including a new method to suppress transmission effects, are explained. Measurements on three model systems which were studied to validate the new technique are presented and compared to simulations.




Electroluminescence from Plasmonic Excitations in a Scanning Tunnelling Microscope


Book Description

This work presents the design and commissioning of a new low-temperature Scanning Tunnelling Microscope equipped with an innovative light collection setup using an integrated, micro-fabricated mirror tip. Commissioning experiments demonstrate the capabilities of this new instrument and reproduce known effects regarding gap plasmons on noble-metal surfaces. Furthermore, different contrasts in the plasmon-mediated light emission from Cobalt nano-islands on a Copper (111) substrate are reported.







Quantum Tunneling of Josephson Vortices in High-Impedance Long Junctions


Book Description

In the last decades, superconducting devices have emerged as a promising platform for quantum technologies, including quantum sensing and quantum computing. Their key elements are Josephson junctions, which allow for coherent supercurrent tunneling between two weakly linked superconductors. If such a junction is extended in one direction to a long junction, the superconducting phase difference can vary in space and time and may allow for quantized phase windings that drive supercurrent vortices.




Light Emission from Single Self-decoupled Molecules in a Scanning Tunnelling Microscope


Book Description

In this work, a clear pathway is presented to achieve well-defined electronically decoupled chromophores from metallic leads without requiring additional insulating layers. To study such self-decoupled molecules, STM equipped with an efficient light detection setup has been used. Results show that the chromophores mounted on tripodal molecular platforms adsorbed on a gold surface present well-defined and efficient electroluminescence down to the single-molecule level.




Quantum Sensing Experiments with Superconducting Qubits


Book Description

Quantum sensing is a vast and emerging field enabling in-situ studies of quantum systems and hence the development of quantum hybrid systems. This work creates the fundament of direct superconducting-magnetic hybrid systems by developing a local microwave sensing scheme and studying the influence of a static magnetic field on a superconducting qubit. Finally, a proof-of-principle hybrid system is demonstrated, which opens the path towards superconducting-magnetic quantum circuits.