Sediment and Radionuclide Transport in Rivers. Summary Report, Field Sampling Program for Cattaraugus and Buttermilk Creeks, New York


Book Description

A three-phase field sampling program was conducted on the Buttermilk-Cattaraugus Creek system to investigate the transport of radionuclides in surface waters as part of a continuing program to provide data for application and verification of Pacific Northwest Laboratory's (PNL) sediment and radionuclide transport model, SERATRA. Phase 1 of the sampling program was conducted during November and December 1977; Phase 2 during September 1978; and Phase 3 during April 1979. Bed sediment, suspended sediment, and water samples were collected over a 45-mile reach of the creek system. Bed sediment samples were also collected at the mouth of Cattaraugus Creek in Lake Erie. A fourth sampling trip was conducted during May 1980 to obtain supplementary channel geometry data and flood plain sediment samples. Radiological analysis of these samples included gamma ray spectrometry analysis, and radiochemical separation and analysis of Sr-90, Pu-238, Pu-239,240, Am-241 and Cm-244. Tritium analysis was also performed on water samples. Based on the evaluation of radionuclide levels in Cattaraugus and Buttermilk Creeks, the Nuclear Fuel Services facility at West Valley, New York, may be the source of Cs-137, Sr-90, CS-134, Co-60, Pu-238, Pu-239,240, Am-241, Cm-244 and tritium found in the bed sediment, suspended sediment and water of Buttermilk and Cattaraugus Creeks.

























Sediment and Radionuclide Transport in Rivers


Book Description

This report describes FY-1979 analysis results on flow, sediment and radionuclide data collected in Cattaraugus, Buttermilk and Franks Creek, New York. The objective of the study is to investigate the radionuclide transport in these streams as a part of a continuing program to provide data required for application and verification of the Sediment and Radionuclide Transport Model (SERATRA). Radiological analyses were performed on sand, silt and clay size fractions of suspended and bed sediment, as well as for dissolved radionuclides. These include gamma-ray emitters plus 9°Sr, 238Pu, 239{sup }−{sup }24°Pu, 241Am, 244Cm and 3H. Among radionuclides analyzed to date, a principal radionuclide found in the study area is 137Cs. Distributions of 137Cs associated with suspended and bed sediments have sharp peaks at the mouth of the Franks Creek, revealing the contribution of 137Cs from the NFS site. Concentration of 137Cs associated with a clay size fraction of suspended and bed sediments at the mouth of Franks Creek were 32.5 ± 1.5 and 134.0 ± 0.90 pCi/g, respectively. Cesium-134 and cobalt-60 associated with the bed sediment also have higher peaks at the mouth of Franks Creek. However, dissolved and particulate concentrations of other radionuclides analyzed under this study were generally very low and there is no clear evidence to indicate that these radionculides detected in this study area originated from the Nuclear Fuel Service site.