Accelerator Transmutation of Nuclear Waste


Book Description

Researchers at Los Alamos have been developing transmutation concepts involving accelerator-driven nuclear systems. A medium energy, high current proton beam strikes a heavy metal target, producing a high flux of spallation neutrons. These neutrons are moderated to near-thermal energies in a blanket surrounding the target. Materials to be transmuted flow through the blanket region where they are fissioned or transmuted to stable nuclides. Stable or short-lived nuclides are separated while the long-lived radioactive species are returned to the blanket. For most applications the fission energy produced is much greater than that required to power the accelerator and can be directed to the commercial power grid. A number of possible applications are envisioned for accelerator-driven nuclear systems. These include destruction of surplus weapons-grade plutonium, production of tritium, transmutation of commercial spent fuel, and even commercial power generation in next-generation nuclear power plants. Some of these applications will be discussed with particular emphasis on the required chemical separations for such systems.




Status of Accelerator Driven Systems Research and Technology Development


Book Description

One of the greatest challenges for nuclear energy is how to properly manage the highly radioactive waste generated during irradiation in nuclear reactors. Accelerator Driven Systems (ADSs) may offer new prospects and advantages for the transmutation of such high level nuclear waste. ADS or accelerator driven transmutation of waste (ATW) consists of a high power proton accelerator, a heavy metal spallation target that produces neutrons when bombarded by the high power beam, and a sub-critical core that is neutronically coupled to the spallation target. This publication provides a comprehensive state of the art of the ADS technology by representing the different ADS concepts proposed worldwide in the last 15 years, as well as the related R&D activities and demonstration initiatives carried out at national international level.




Nuclear Wastes


Book Description

Disposal of radioactive waste from nuclear weapons production and power generation has caused public outcry and political consternation. Nuclear Wastes presents a critical review of some waste management and disposal alternatives to the current national policy of direct disposal of light water reactor spent fuel. The book offers clearcut conclusions for what the nation should do today and what solutions should be explored for tomorrow. The committee examines the currently used "once-through" fuel cycle versus different alternatives of separations and transmutation technology systems, by which hazardous radionuclides are converted to nuclides that are either stable or radioactive with short half-lives. The volume provides detailed findings and conclusions about the status and feasibility of plutonium extraction and more advanced separations technologies, as well as three principal transmutation concepts for commercial reactor spent fuel. The book discusses nuclear proliferation; the U.S. nuclear regulatory structure; issues of health, safety and transportation; the proposed sale of electrical energy as a means of paying for the transmutation system; and other key issues.




Nuclear Methods For Transmutation Of Nuclear Waste: Problems, Perspectives, Cooperative Research - Proceedings Of The International Workshop


Book Description

Long-lived radioactive materials from the operation of nuclear power plants and from the maintenance and decommissioning of nuclear weapons pose environmental and security risks. Technologies that would counter such risks are under intense study worldwide. One such technology, transmutation by nuclear means into shorter-lived materials, was the subject of an international workshop in Russia, where the need for a viable solution of this problem is particularly strong.Current problems of that technology and future perspectives and cooperative research possibilities involving Russian and East European facilities are discussed by scientists from Russia, the United States and seven other countries representing basic research institutes, former nuclear weapons laboratories and nuclear industries. Computer modeling, data bases and experimental investigations needed for the conceptualization of demonstration, prototype and production facilities are treated in detail. Progress on the planning and construction of the first demonstration facilities is also described.From these proceedings it becomes evident that the problems inherent in radioactive waste accumulation can be solved only by international cooperation in which conventional methods are supplemented by new technologies, and that such a solution may require a sustained effort comparable to the Manhattan Project and the analogous project in the former USSR at the beginning of the nuclear era.




Nuclear Back-end and Transmutation Technology for Waste Disposal


Book Description

This book covers essential aspects of transmutation technologies, highlighting especially the advances in Japan. The accident at the Fukushima Daiichi Nuclear Power Plant (NPP) has caused us to focus attention on a large amount of spent nuclear fuels stored in NPPs. In addition, public anxiety regarding the treatment and disposal of high-level radioactive wastes that require long-term control is growing. The Japanese policy on the back-end of the nuclear fuel cycle is still unpredictable in the aftermath of the accident. Therefore, research and development for enhancing the safety of various processes involved in nuclear energy production are being actively pursued worldwide. In particular, nuclear transmutation technology has been drawing significant attention after the accident. This publication is timely with the following highlights: 1) Development of accelerator-driven systems (ADSs), which is a brand-new reactor concept for transmutation of highly radioactive wastes; 2) Nuclear reactor systems from the point of view of the nuclear fuel cycle. How to reduce nuclear wastes or how to treat them including the debris from TEPCO’s Fukushima nuclear power stations is discussed; and 3) Environmental radioactivity, radioactive waste treatment and geological disposal policy. State-of-the-art technologies for overall back-end issues of the nuclear fuel cycle as well as the technologies of transmutation are presented here. The chapter authors are actively involved in the development of ADSs and transmutation-related technologies. The future of the back-end issues in Japan is very uncertain after the accident at the Fukushima Daiichi NPP and this book provides an opportunity for readers to consider the future direction of those issues.




Accelerator-driven Transmutation of High-level Waste from the Defense and Commercial Sectors


Book Description

This is the final report of a three-year, Laboratory-Directed Research and Development (LDRD) project at the Los Alamos National Laboratory (LANL). The major goal has been to develop accelerator transmutation of waste (ATW) system designs that will thoroughly and rapidly transmute nuclear waste, including plutonium from dismantled weapons and spent reactor fuel, while generating useful electrical power and without producing a long-lived radioactive waste stream. We have identified and quantified the unique qualities of subcritical nuclear systems and their capabilities in bringing about the complete destruction of plutonium. Although the 1191 subcritical systems involved in our most effective designs radically depart from traditional nuclear reactor concepts, they are based on extrapolations of existing technologies. Overall, care was taken to retain the highly desired features that nuclear technology has developed over the years within a conservative design envelope. We believe that the ATW systems designed in this project will enable almost complete destruction of nuclear waste (conversion to stable species) at a faster rate and without many of the safety concerns associated with the possible reactor approaches.







Transmutation of High-level Radioactive Waste and Production of 233U Using an Accelerator-driven Reactor


Book Description

Reactor safety, the disposal of high-level nuclear waste, and nonproliferation of nuclear material for military purposes are the problems of greatest concern for nuclear energy. Technologies for accelerators developed in the field of high-energy physics can contribute to solving these problems. For reactor safety, especially for that of a Na-cooled fast reactor, the use of an accelerator, even a small one, can enhance the safety using a slightly subcritical reactor. There is growing concern about how we can deal with weapons-grade Pu, and about the large amount of Pu accumulating from the operation of commercial reactors. It has been suggested that this Pu could be incinerated, using the reactor and a proton accelerator. However, because Pu is a very valuable material with future potential for generating nuclear energy, we should consider transforming it into a proliferation-resistant material that cannot be used for making bombs, rather than simply eliminating the Pu. An accelerator-driven fast reactor (700 MWt), run in a subcritical condition, and fueled with MOX can generate 233U more safely and efficiently than can a critical reactor. We evaluate the production of 233U, 239Pu, and the transmutation of the long-lived fission products of 99Tc and 129I, which are loaded with YH{sub 1.7} between the fast core and blanket, by reducing the conversion factor of Pu to 233U. And we assessed the rates of radiation damage, hydrogen production, and helium production in a target window and in the surrounding vessel.




Radiation Safety of Accelerator Based Radioisotope Production Facilities


Book Description

Radioisotopes are used worldwide in a range of medical, industrial, research and academic applications. A large proportion of these radioisotopes are produced in particle accelerators, and the number of institutions that operate linear accelerators or cyclotrons and manufacture and distribute radiopharmaceuticals, for example, is significant and increasing. The production of radioisotopes using particle accelerators poses significant radiation hazards to workers, members of the public, and the environment when accelerators are operated without adequate radiation safety measures. This Safety Guide provides practical guidance for implementing radiation protection and safety measures in such facilities involved in the production and use of radioisotopes.




Advanced Nuclear Energy Systems Toward Zero Release of Radioactive Wastes


Book Description

This volume is a collection of the papers presented at the International Seminar on Advanced Nuclear Energy Systems toward Zero Release of Radioactive Wastes, which was held in Japan in November 2000. Scientists and engineers working in academia, research organizations and industry came together to discuss the role and contributions of nuclear energy to the environmental issues in the new millennium. It provided a forum for open discussions about the pursuit of solutions for the reduction of nuclear wastes based on the accelerator and fusion technologies, in addition to the advanced fission technology to harmonize the nuclear energy systems with the global environment. It also promoted future international collaboration in the following research fields: the role of nuclear energy in the new millennium; waste management; transmutation of minor actinides and fission products; advanced fission systems, accelerator driven systems, fusion systems, nuclear database, and advanced nuclear fuel cycles for transmutation of wastes. Published originally as a special issue (volume 40/3-4) of the international journal Progress in Nuclear Energy.