Nuclear Wastes


Book Description

Disposal of radioactive waste from nuclear weapons production and power generation has caused public outcry and political consternation. Nuclear Wastes presents a critical review of some waste management and disposal alternatives to the current national policy of direct disposal of light water reactor spent fuel. The book offers clearcut conclusions for what the nation should do today and what solutions should be explored for tomorrow. The committee examines the currently used "once-through" fuel cycle versus different alternatives of separations and transmutation technology systems, by which hazardous radionuclides are converted to nuclides that are either stable or radioactive with short half-lives. The volume provides detailed findings and conclusions about the status and feasibility of plutonium extraction and more advanced separations technologies, as well as three principal transmutation concepts for commercial reactor spent fuel. The book discusses nuclear proliferation; the U.S. nuclear regulatory structure; issues of health, safety and transportation; the proposed sale of electrical energy as a means of paying for the transmutation system; and other key issues.




Optimization of Accelerator-driven Technology for LWR Waste Transmutation


Book Description

The role of accelerator-driven transmutation technology is examined in the context of the destruction of actinide waste from commercial light water reactors. It is pointed out that the commercial plutonium is much easier to use for entry-level nuclear weapons than weapons plutonium. Since commercial plutonium is easier to use, since there is very much more of it already, and since it is growing rapidly, the permanent disposition of commercial plutonium is an issue of greater importance than weapons plutonium. The minor actinides inventory, which may be influenced by transmutation, is compared in terms of nuclear properties with commercial and weapons plutonium and for possible utility as weapons material. Fast and thermal spectrum systems are compared as means for destruction of plutonium and the minor actinides. it is shown that the equilibrium fast spectrum actinide inventory is about 100 times larger than for thermal spectrum systems, and that there is about 100 times more weapons-usable material in the fast spectrum system inventory compared to the thermal spectrum system. Finally it is shown that the accelerator size for transmutation can be substantially reduced by design which uses the accelerator-produced neutrons only to initiate the unsustained fission chains characteristic of the subcritical system. The analysis argues for devoting primary attention to the development of thermal spectrum transmutation technology. A thermal spectrum transmuter operating at a fission power of 750-MWth fission power, which is sufficient to destroy the actinide waste from one 3,000-MWth light water reactor, may be driven by a proton beam of 1 GeV energy and a current of 7 mA. This accelerator is within the range of realizable cyclotron technology and is also near the size contemplated for the next generation spallation neutron source under consideration by the US, Europe, and Japan.










Target and Core Optimization for an Electron Accelerator-Driven Transmutation Facility


Book Description

The current statutory limit for Yucca Mountain is quickly being met by waste produced at the reactors operating in the United States. A possible method of modifying reactor waste for more efficient storage in Yucca Mountain is transmutation. This study analyzes the use of an electron accelerator targeting its beam on a neutron producing target within a subcritical reactor fueled with transuranic waste from power reactor operations. To maximize the transmutation effectiveness of the design, several loading patterns were analyzed for neutronics behavior and transmutation effectiveness. Designs utilizing multiple batches of fuel or multiple targets within the core were also analyzed. The loading pattern analysis showed no clear beneficial loading pattern for the neutronics of the core; however, the results indicated that placing Curium within the innermost fuel assemblies improved the transmutation effectiveness of the core. The most effective loading pattern in terms of neutronics and transmutation effectiveness utilized Curium assemblies in the innermost locations, Americium assemblies in the second ring, and Neptunium and Plutonium assemblies in the outermost locations. The use of multiple batches in the core layout demonstrated superior neutronics behavior but lacked in transmutation effectiveness. On the other hand, the use of multiple targets in the core did not exhibit the lower peaking factors expected and also performed poorly in the area of transmutation effectiveness. Most likely, these core designs should be combined with more effective loading patterns to maximize their benefits. When comparing electron accelerator based systems with proton accelerator based systems, the proton based systems have a significant advantage due to the higher neutron production efficiency within the target. However, economic and timeline considerations make the deployment of electron based systems attractive in specific scenarios.




ATW Neutronics Design Studies


Book Description

The Accelerator Transmutation of Waste (ATW) concept has been proposed as a transuranics (TRU) (and long-lived fission product) incinerator for processing the 87,000 metric tonnes of Light Water Reactor used fuel which will have been generated by the time the currently deployed fleet of commercial reactors in the US reach the end of their licensed lifetime. The ATW is proposed to separate the uranium from the transuranics and fission products in the LWR used fuel, to fission the transuranics, to send the LWR and ATW generated fission products to the geologic repository and to send the uranium to either a low level waste disposal site or to save it for future use. The heat liberated in fissioning the transuranics would be converted to electricity and sold to partially offset the cost of ATW construction and operations. Options for incineration of long-lived fission products are under evaluation. A six-year science-based program of ATW trade and system studies was initiated in the US FY 2000 to achieve two main purposes: (1) ''to evaluate ATW within the framework of nonproliferation, waste management, and economic considerations, '' and (2) ''to evaluate the efficacy of the numerous technical options for ATW system configuration.'' This paper summarizes the results from neutronics and thermal/hydraulics trade studies which were completed at Argonne National Laboratory during the first year of the program. Core designs were developed for Pb-Bi cooled and Na cooled 840 MW{sub th} fast spectrum transmuter designs employing recycle. Additionally, neutronics analyses were performed at Argonne for a He cooled 600 MW{sub th} hybrid thermal and fast core design proposed by General Atomics Co. which runs critical for 3/4 and subcritical for 1/4 of its four year once-thin burn cycle. The mass flows and the ultimate loss of transuranic isotopes to the waste stream per unit of heat generated during transmutation have been calculated on a consistent basis and are compared. (Long-lived fission product incineration has not been considered in the studies reported here.).







日本の歴史


Book Description




A Study on the Feasibility of Electron-based Accelerator Driven Systems for Nuclear Waste Transmutation


Book Description

Nuclear waste transmutation is an important option for the development of advanced fuel cycle and effective nuclear waste management. The electron accelerator driven system (ADS) was investigated in the study for nuclear waste transmutation as an alternative to proton based ADS. Target design and optimization was carried out to obtain maximum neutron generation. Subcritical core design based on single and multiple targets was investigated. System performance between electron-based ADS and proton-based ADS was compared in terms of neutron generation rate, transmutation efficiency and power generation. It was determined that the electron-based target was capable of providing high neutron flux, small target geometry size, small scale subcritical core, and low radiation damage. Multiple target design in the electron-driven ADS was also explored to flatten power distribution in the ADS subcritical core. Regarding transmutation, the power peaking factors in both the electron- and proton- ADS increase ~ 10% during the burnup period of 700 days. Thermal power in proton ADS is higher than that of electron ADS by a factor ~ 20. The transmutation effectiveness of preliminary electron-based ADS is smaller by a factor of 11 compared to preliminary proton-based ADS. Proton ADS has higher radiation damage to target materials and surrounding materials. The capital cost for electron-based and proton-based accelerator facility is fairly comparable with the cost of proton-based facilities being slightly higher by a factor of 20%. Comparing with the proton-driven ADS, the electron-driven ADS pros include small target size and small core scale, multiple target possibility for low PPF, low radiation damage to target surroundings, wide availability electron beam at ~100 MeV, and low capital cost of electron accelerator facility. There are also aspects against electron-driven ADS, including low efficiency of neutron generation rate, low transmutation efficiency, low thermal power, and elec.