Book Description
When aerosols enter the atmosphere through anthropogenic and natural activities, they interact with clouds in the atmosphere in what is termed aerosol-cloud interactions (ACI). ACI alter the cloud's radiative properties by acting as cloud condensation nuclei within the cloud, thereby reducing the mean drop size and increasing the cloud's albedo and cooling the earth by reflecting incoming shortwave radiation in what is termed the first indirect effect. By reducing the mean drop size throughout the cloud, aerosol also act to delay precipitation formation, leading to larger, longer lived clouds and further cooling the earth in a process known as the second indirect effect. Using four years of satellite observations, the overall impact of aerosols on warm cloud radiative effect is evaluated. Warm clouds are defined as clouds with cloud top temperatures below freezing level. The estimates are constrained within regimes of stability, relative humidity of the free atmosphere, and by the scene liquid water path to control for how meteorology modulates the strength and sign of ACI. The sum of the first and second indirect effect, estimates of how aerosols alter the warm cloud shortwave effect and cloud fraction, are compared to an estimate of the full indirect effect, which includes all changes to the warm cloud shortwave radiative effect. The decomposed, or summative, indirect effect (-0.26 +/- .15 Wm2) is less than the full indirect effect (-0.32 +/- .16 Wm2), though they lie within each other's uncertainty estimates. When the decomposed indirect effect is further constrained by precipitation, the estimate decreases to .21 +/- .15 Wm2. The difference between the full indirect effect forcing and the decomposed forcings may be secondary indirect effects not included in our decomposition. The second indirect effect includes not only the cloud extent broadening, but the cloud depth increasing. This deepening response may increase warming due to a larger longwave cloud radiative effect. The longwave indirect effect susceptibility is decomposed to determine how large it may potentially be and whether it could offset any cooling due to the shortwave indirect effect. We find the longwave indirect effect does have the potential to offset cooling through cloud deepening in regions where the shortwave indirect effect is extremely small, however the magnitude of the longwave component is sensitive to the diurnal cycle. Cloud deepening signals clouds may be invigorated, or experiencing a state where precipitation formation and turbulence increase due to ACI. The effects of aerosol on precipitation formation and vertical motion are investigated using WALRUS, an algorithm of latent heating within the cloud determined using CloudSat radar returns. The LWP is constrained to thicker clouds 150 gm2